My impression of the weapon was that the gas was used to 'c.o.c.k.' the weapon, not propel the bolt. Still, even if possible to engineer, the gas canister in the stock of the weapon would only have enough gas to 'cycle' the action a few times before pressure was too low to c.o.c.k. the weapon.... assuming of course that you could ever get enough pressure to c.o.c.k. a crossbow (which tend to be in the 100 - 150 lb pull category for modern crossbows).
Basically impossible given the canister size and the size of the crossbow. Still, cool as hell for visual effects.
Edit: damn language filter